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000917542 1001_ $$00000-0003-3261-5846$$aRen, Yaoyu$$b0
000917542 245__ $$aOxide‐Based Solid‐State Batteries: A Perspective on Composite Cathode Architecture
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000917542 520__ $$aAbstract: “Oxide-Based Solid-State Batteries: A Perspective on Composite Cathode Architecture”The garnet-type phase Li7La3Zr2O12 (LLZO) attracts significant attention as an oxide solid electrolyte to enable safe and robust solid-state batteries (SSBs) with potentially high energy density. However, while significant progress has been made in demonstrating compatibility with Li metal, integrating LLZO into composite cathodes remains a challenge. The current perspective focuses on the critical issues that need to be addressed to achieve the ultimate goal of an all-solid-state LLZO-based battery that delivers safety, durability, and pack-level performance characteristics that are unobtainable with state-of-the-art Li-ion batteries. This perspective complements existing reviews of solid/solid interfaces with more emphasis on understanding numerous homo- and heteroionic interfaces in a pure oxide-based SSB and the various phenomena that accompany the evolution of the chemical, electrochemical, structural, morphological, and mechanical properties of those interfaces during processing and operation. Finally, the insights gained from a comprehensive literature survey of LLZO–cathode interfaces are used to guide efforts for the development of LLZO-based SSBs.
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000917542 7001_ $$00000-0003-2336-6059$$aDanner, Timo$$b1
000917542 7001_ $$00000-0002-4402-5432$$aMoy, Alexandra$$b2
000917542 7001_ $$0P:(DE-Juel1)145623$$aFinsterbusch, Martin$$b3
000917542 7001_ $$00000-0002-9312-930X$$aHamann, Tanner$$b4
000917542 7001_ $$aDippell, Jan$$b5
000917542 7001_ $$aFuchs, Till$$b6
000917542 7001_ $$aMüller, Marius$$b7
000917542 7001_ $$aHoft, Ricky$$b8
000917542 7001_ $$00000-0003-1744-3732$$aWeber, André$$b9
000917542 7001_ $$00000-0001-8855-8006$$aCurtiss, Larry A.$$b10
000917542 7001_ $$00000-0003-0570-9169$$aZapol, Peter$$b11
000917542 7001_ $$aKlenk, Matthew$$b12
000917542 7001_ $$aNgo, Anh T.$$b13
000917542 7001_ $$00000-0003-2217-6392$$aBarai, Pallab$$b14
000917542 7001_ $$aWood, Brandon C.$$b15
000917542 7001_ $$00000-0002-5007-4249$$aShi, Rongpei$$b16
000917542 7001_ $$00000-0002-5391-0804$$aWan, Liwen F.$$b17
000917542 7001_ $$aHeo, Tae Wook$$b18
000917542 7001_ $$aEngels, Martin$$b19
000917542 7001_ $$00000-0002-6875-0057$$aNanda, Jagjit$$b20
000917542 7001_ $$00000-0002-6587-7757$$aRichter, Felix H.$$b21
000917542 7001_ $$00000-0003-1449-8172$$aLatz, Arnulf$$b22
000917542 7001_ $$aSrinivasan, Venkat$$b23
000917542 7001_ $$00000-0002-9221-4756$$aJanek, Jürgen$$b24
000917542 7001_ $$00000-0002-3099-462X$$aSakamoto, Jeff$$b25
000917542 7001_ $$00000-0002-0667-1927$$aWachsman, Eric D.$$b26
000917542 7001_ $$0P:(DE-Juel1)171780$$aFattakhova-Rohlfing, Dina$$b27$$eCorresponding author
000917542 773__ $$0PERI:(DE-600)2594556-7$$a10.1002/aenm.202201939$$gVol. 13, no. 1, p. 2201939 -$$n1$$p2201939 -$$tAdvanced energy materials$$v13$$x1614-6832$$y2023
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