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@ARTICLE{Zhang:1017656,
author = {Zhang, Shidong and Yu, Shangzhe and Peters, Roland and
Beale, Steven B. and Marschall, Holger and Kunz, Felix and
Eichel, Rüdiger-A.},
title = {{A} new procedure for rapid convergence in numerical
performance calculations of electrochemical cells},
journal = {Electrochimica acta},
volume = {472},
issn = {0013-4686},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2023-04272},
pages = {143275 -},
year = {2023},
abstract = {This paper introduces a novel coupled region-to-region
numerical procedure for electric field potential
calculations. A conventional segregated scheme is also
introduced to illustrate the coupling issues that exist in
performance calculations in electrochemical devices.
Numerical simulations are conducted for a solid oxide cell
operating in both fuel cell and electrolysis modes. The cell
performance is predicted with both segregated and coupled
methods. A comparison between the coupled and segregated
schemes shows that the former greatly outperforms the
latter, reducing convergence times (from 5000 to 300
iterations) and improving stability. A smaller coupling
coefficient contributes to the convergence as well, however,
less markedly. The coupled region-to-region approach may
readily be applied to numerous other scenarios, e.g., heat
transfer problems between multiple phases and regions.},
cin = {IEK-9},
ddc = {540},
cid = {I:(DE-Juel1)IEK-9-20110218},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) / HITEC -
Helmholtz Interdisciplinary Doctoral Training in Energy and
Climate Research (HITEC) (HITEC-20170406)},
pid = {G:(DE-HGF)POF4-1231 / G:(DE-Juel1)HITEC-20170406},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001105536100001},
doi = {10.1016/j.electacta.2023.143275},
url = {https://juser.fz-juelich.de/record/1017656},
}