TypAmountVATCurrencyShareStatusCost centre
Hybrid-OA3530.000.00EUR100.00 %(Zahlung angewiesen)E6610009
Sum3530.000.00EUR   
Total3530.00     
Journal Article FZJ-2023-04272

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A new procedure for rapid convergence in numerical performance calculations of electrochemical cells

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2023
Elsevier New York, NY [u.a.]

Electrochimica acta 472, 143275 - () [10.1016/j.electacta.2023.143275]

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Abstract: This paper introduces a novel coupled region-to-region numerical procedure for electric field potential calculations. A conventional segregated scheme is also introduced to illustrate the coupling issues that exist in performance calculations in electrochemical devices. Numerical simulations are conducted for a solid oxide cell operating in both fuel cell and electrolysis modes. The cell performance is predicted with both segregated and coupled methods. A comparison between the coupled and segregated schemes shows that the former greatly outperforms the latter, reducing convergence times (from 5000 to 300 iterations) and improving stability. A smaller coupling coefficient contributes to the convergence as well, however, less markedly. The coupled region-to-region approach may readily be applied to numerous other scenarios, e.g., heat transfer problems between multiple phases and regions.

Classification:

Contributing Institute(s):
  1. Grundlagen der Elektrochemie (IEK-9)
Research Program(s):
  1. 1231 - Electrochemistry for Hydrogen (POF4-123) (POF4-123)
  2. HITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406) (HITEC-20170406)

Appears in the scientific report 2023
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Medline ; Creative Commons Attribution CC BY 4.0 ; OpenAccess ; Clarivate Analytics Master Journal List ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; Essential Science Indicators ; IF >= 5 ; JCR ; NationallizenzNationallizenz ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection
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 Record created 2023-11-03, last modified 2024-07-12


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