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001020973 1001_ $$0P:(DE-Juel1)186842$$aYan, Peng$$b0$$ufzj
001020973 245__ $$aBlended Salt Electrolyte Design for Enhanced NMC811||Graphite Cell Performance
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001020973 520__ $$aThe high energy density, nickel-rich layered cathode material LiNi0.8Mn0.1Co0.1O2(NMC811) is recognized as a promising candidate for next-generation batterychemistries. However, due to their structural and interfacial instability, nickel-richNMC cathodes still face a number of challenges in practical application. For thisreason, the design and development of novel electrolyte formulations, able tostabilize the nickel-rich cathode|electrolyte interface, are highly demanded. In thiswork, a novel electrolyte is developed using lithium (difluoromethanesulfonyl)(trifluoromethanesulfonyl)imide (LiDFTFSI) and lithium hexafluorophosphate(LiPF6) as salt blend in an organic carbonate-solvent based solvent mixture. Thepresence of LiDFTFSI notably enhances the electrochemical performance of theresulting NMC811||graphite cells. Further advancement of the considered cellchemistry is achieved by introducing the well-known functional electrolyteadditive vinylene carbonate (VC), which was found to feature a synergistic effectwith LiDFTFSI. The formation of a homogenous, effective, and robust solidelectrolyte interphase (SEI) as well as cathode electrolyte interphase (CEI) on thecorresponding electrodes resulted in superior electrochemical performance.
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001020973 7001_ $$0P:(DE-HGF)0$$aShevchuk, Mykhailo$$b1
001020973 7001_ $$0P:(DE-Juel1)176954$$aWölke, Christian$$b2$$ufzj
001020973 7001_ $$0P:(DE-Juel1)188450$$aPfeiffer, Felix$$b3$$ufzj
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001020973 7001_ $$0P:(DE-HGF)0$$aBaghernejad, Masoud$$b5
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001020973 7001_ $$0P:(DE-Juel1)166130$$aWinter, Martin$$b7$$ufzj
001020973 7001_ $$0P:(DE-Juel1)171204$$aCekic-Laskovic, Isidora$$b8$$eCorresponding author
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