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@ARTICLE{Yan:1020973,
      author       = {Yan, Peng and Shevchuk, Mykhailo and Wölke, Christian and
                      Pfeiffer, Felix and Berghus, Debbie and Baghernejad, Masoud
                      and Röschenthaler, Gerd-Volker and Winter, Martin and
                      Cekic-Laskovic, Isidora},
      title        = {{B}lended {S}alt {E}lectrolyte {D}esign for {E}nhanced
                      {NMC}811||{G}raphite {C}ell {P}erformance},
      journal      = {Small structures},
      volume       = {5},
      number       = {4},
      issn         = {2688-4062},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-00433},
      pages        = {2300425},
      year         = {2024},
      abstract     = {The high energy density, nickel-rich layered cathode
                      material LiNi0.8Mn0.1Co0.1O2(NMC811) is recognized as a
                      promising candidate for next-generation batterychemistries.
                      However, due to their structural and interfacial
                      instability, nickel-richNMC cathodes still face a number of
                      challenges in practical application. For thisreason, the
                      design and development of novel electrolyte formulations,
                      able tostabilize the nickel-rich cathode|electrolyte
                      interface, are highly demanded. In thiswork, a novel
                      electrolyte is developed using lithium
                      (difluoromethanesulfonyl)(trifluoromethanesulfonyl)imide
                      (LiDFTFSI) and lithium hexafluorophosphate(LiPF6) as salt
                      blend in an organic carbonate-solvent based solvent mixture.
                      Thepresence of LiDFTFSI notably enhances the electrochemical
                      performance of theresulting NMC811||graphite cells. Further
                      advancement of the considered cellchemistry is achieved by
                      introducing the well-known functional electrolyteadditive
                      vinylene carbonate (VC), which was found to feature a
                      synergistic effectwith LiDFTFSI. The formation of a
                      homogenous, effective, and robust solidelectrolyte
                      interphase (SEI) as well as cathode electrolyte interphase
                      (CEI) on thecorresponding electrodes resulted in superior
                      electrochemical performance.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / BIG-MAP -
                      Battery Interface Genome - Materials Acceleration Platform
                      (957189) / BATTERY 2030PLUS - BATTERY 2030+ large-scale
                      research initiative: At the heart of a connected green
                      society (957213)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(EU-Grant)957189 /
                      G:(EU-Grant)957213},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001130274600001},
      doi          = {10.1002/sstr.202300425},
      url          = {https://juser.fz-juelich.de/record/1020973},
}