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Total1512.00     
Journal Article FZJ-2024-05321

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Connecting Cell Structure and Current‐Dependent Environment Changes in CO2 Electrolysis to GDE Operation Regimes and Multi‐Cell Interaction

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2024
Wiley-VCH Verlag GmbH Weinheim

Electrochemical science advances e202400013, e202400013 () [10.1002/elsa.202400013]

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Abstract: Consecutive development of materials, components, and ultimately, devices does not appear to be a promising strategy in CO2 electroreduction because maintaining comparability and transferring results between idealized and application-oriented systems proves challenging. A modular cell design and tracking cell conditions via sensors may be a solution. We displayed a strategy to characterize gas diffusion electrode operating regimes in a flow cell with regard to different current density ranges, as well as the impact of the flow gap design. We revealed strong interdependencies between cell components, their functions as well as individual cells when integrated into a stack. Expanding the scope and resolution of experimental data made new information on the change of system parameters in flow cells accessible.

Keyword(s): Chemical Reactions and Advanced Materials (1st) ; Energy (1st) ; Chemistry (2nd)

Classification:

Contributing Institute(s):
  1. Grundlagen der Elektrochemie (IET-1)
Research Program(s):
  1. 1232 - Power-based Fuels and Chemicals (POF4-123) (POF4-123)
  2. iNEW2.0 - Verbundvorhaben iNEW2.0: Im Zentrum des Inkubators Nachhaltige Elektrochemische Wertschöpfungsketten (iNEW 2.0) steht die Erforschung und Entwicklung neuartiger und leistungsfähiger Elektrolyse-verfahren zur Anwendung in nachhaltigen Power-to-X (P2X) Wertschöpfungsketten. (BMBF-03SF0627A) (BMBF-03SF0627A)
  3. HITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406) (HITEC-20170406)

Appears in the scientific report 2024
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Medline ; Creative Commons Attribution CC BY 4.0 ; DOAJ ; OpenAccess ; Article Processing Charges ; DOAJ Seal ; Ebsco Academic Search ; Fees
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Open Access

 Datensatz erzeugt am 2024-08-30, letzte Änderung am 2025-10-27


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