Journal Article PreJuSER-12812

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png
Reaction-controlled diffusion

 ;  ;

2000
APS College Park, Md.

Physical review / E 62(5), 6071-6077 () [10.1103/PhysRevE.62.6071]

This record in other databases:    

Please use a persistent id in citations:   doi:

Abstract: The dynamics of a coupled two-component nonequilibrium system is examined by means of continuum field theory representing the corresponding master equation. Particles of species A may perform hopping processes only when particles of different type B are present in their environment. Species B is subject to diffusion-limited reactions. If the density of B particles attains a finite asymptotic value (active state), the A species displays normal diffusion. On the other hand, if the B density decays algebraically proportional tot(-alpha) at long times (inactive state), the effective attractive A-B interaction is weakened. The combination of B decay and activated A hopping processes gives rise to anomalous diffusion, with mean-square displacement ((x) over right arrow (A)(t)(2)) proportional to t(1-alpha) for alpha <1. Such algebraic subdiffusive behavior ensues for nth-order B annihilation reactions (nB-->O) with n greater than or equal to 3, and n = 2 for d<2. The mean-square displacement of the A particles grows only logarithmically with time in the case of B pair annihilation (n = 2) and d<greater than or equal to>2 dimensions. For radioactive B decay (n = 1), the A particles remain localized. If the A particles may hop spontaneously as well, or if additional random forces are present, the A-B couplings becomes irrelevant, and conventional diffusion is recovered in the long-time limit.

Keyword(s): J


Note: Record converted from VDB: 12.11.2012

Contributing Institute(s):
  1. Institut für Festkörperforschung (IFF)
Research Program(s):
  1. Polymere, Membranen und komplexe Flüssigkeiten (23.30.0)

Appears in the scientific report 2000
Database coverage:
American Physical Society Transfer of Copyright Agreement ; OpenAccess
Click to display QR Code for this record

The record appears in these collections:
Document types > Articles > Journal Article
Workflow collections > Public records
Publications database
Open Access

 Record created 2012-11-13, last modified 2023-02-17