Journal Article FZJ-2014-00046

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Magnetic structure of superconducting Eu(Fe$_{0.82}$Co$_{0.18}$)$_2$As$_2$ as revealed by single-crystal neutron diffraction

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2013
APS College Park, Md.

Physical review / B 88(21), 214516 () [10.1103/PhysRevB.88.214516]

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Abstract: The magnetic structure of superconducting Eu(Fe$_{0.82}$Co$_{0.18}$)$_2$As$_2$ is unambiguously determined by single-crystal neutron diffraction. A long-range ferromagnetic order of the $Eu^{2+}$ moments along the c direction is revealed below the magnetic phase transition temperature $T_C$=17 K. In addition, the antiferromagnetism of the $Fe^{2+}$ moments still survives and the tetragonal-to-orthorhombic structural phase transition is also observed, although the transition temperatures of the Fe spin-density-wave (SDW) order and the structural phase transition are significantly suppressed to $T_N$=70 K and $T_S$=90 K, respectively, compared to the parent compound EuFe$_2$As$_2$. We present microscopic evidence for the coexistence of the Eu ferromagnetism and the Fe SDW in the superconducting crystal. The superconductivity competes with the Fe SDW in Eu(Fe$_{0.82}$Co$_{0.18}$)$_2$As$_2$. Moreover, the comparison between Eu(Fe$_{1−x}$Co$_x$)$_2$As$_2$ and Ba(Fe$_{1−x}$Co$_x$)$_2$As$_2$ indicates a considerable influence of the rare-earth element Eu on the magnetism of the Fe sublattice.

Keyword(s): Magnetic Materials (1st) ; Key Technologies (1st) ; Information Technology and Functional Materials (1st) ; Magnetism (2nd)

Classification:

Contributing Institute(s):
  1. Streumethoden (PGI-4)
  2. Streumethoden (JCNS-2)
  3. JCNS-FRM-II (JCNS (München) ; Jülich Centre for Neutron Science JCNS (München) ; JCNS-FRM-II)
  4. JARA-FIT (JARA-FIT)
Research Program(s):
  1. 422 - Spin-based and quantum information (POF2-422) (POF2-422)
  2. 424 - Exploratory materials and phenomena (POF2-424) (POF2-424)
  3. 542 - Neutrons (POF2-542) (POF2-542)
  4. 544 - In-house Research with PNI (POF2-544) (POF2-544)
  5. 54G - JCNS (POF2-54G24) (POF2-54G24)
Experiment(s):
  1. Measurement at external facility

Appears in the scientific report 2013
Database coverage:
Medline ; American Physical Society Transfer of Copyright Ag ; OpenAccess ; Current Contents - Social and Behavioral Sciences ; JCR ; NationallizenzNationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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Institute Collections > JCNS > JCNS-FRM-II
Document types > Articles > Journal Article
Institute Collections > JCNS > JCNS-2
JARA > JARA > JARA-JARA\-FIT
Institute Collections > PGI > PGI-4
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 Record created 2014-01-03, last modified 2025-01-29


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