Journal Article PreJuSER-16697

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Spin orientation and sign of the Rashba splitting in Bi/Cu(111)

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2011
APS College Park, Md.

Physical review / B 84(11), 115426 () [10.1103/PhysRevB.84.115426]

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Abstract: Whereas the magnitude of the Rashba spin splitting at surfaces has been studied in detail, less is known about its sign which determines the precise spin orientation of the electronic states. We investigate the microscopic origin of this sign by spin-resolved photoemission experiments and first-principles calculations on the strongly spin-orbit coupled surface states in Bi/Cu(111). We conclude that the sign of the Rashba splitting is determined by the particular charge asymmetry near the atomic cores. The precise spin orientation on heavy-element surfaces thus can comprise information on wave-function localizations and related aspects otherwise hardly accessible by other experimental methods.

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Note: We gratefully acknowledge experimental support by Ryusei Tateishi and Yuta Yamamoto. G.B. would like to thank Hugo Dil for helpful discussions. This work was supported by the Grant-in-Aid for Scientific Research (A) 20244045, the G-COE programs (G-03), the Bundesministerium fur Bildung und Forschung (Grant Nos. 05K10WW1/2 and 05KS1WMB/1), and the Deutsche Forschunsgsgemeinschaft (FOR 1162). H.B. acknowledges support by the Japan Society for the Promotion of Science.

Contributing Institute(s):
  1. Quanten-Theorie der Materialien (PGI-1)
  2. Quanten-Theorie der Materialien (IAS-1)
  3. Jülich-Aachen Research Alliance - Fundamentals of Future Information Technology (JARA-FIT)
  4. Jülich-Aachen Research Alliance - Simulation Sciences (JARA-SIM)
Research Program(s):
  1. Grundlagen für zukünftige Informationstechnologien (P42)

Appears in the scientific report 2011
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 Record created 2012-11-13, last modified 2023-04-26