Journal Article PreJuSER-22289

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Single Molecule and Single Atom Sensors for Atomic Resolution Imaging of Chemically Complex Surfaces

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2011
American Chemical Society Washington, DC

Journal of the American Chemical Society 133(42), 16847 - 16851 () [10.1021/ja204624g]

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Abstract: Individual Xe atoms as well as single CO and CH(4) molecules adsorbed at the tip apex of a scanning tunneling microscope (STM) function as microscopic force sensors that change the tunneling current in response to the forces acting from the surface. An STM equipped with any of these sensors is able to image the short-range Pauli repulsion and thus resolve the inner structure of large organic adsorbate molecules. Differences in the performance of the three studied sensors suggest that the sensor functionality can be tailored by tuning the interaction between the sensor particle and the STM tip.

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Note: We thank M. Sokolowski (Bonn) for helpful discussions. R.T. acknowledges support by the Helmholtz-Gemeinschaft.

Contributing Institute(s):
  1. Funktionale Nanostrukturen an Oberflächen (PGI-3)
  2. Jülich-Aachen Research Alliance - Fundamentals of Future Information Technology (JARA-FIT)
Research Program(s):
  1. Grundlagen für zukünftige Informationstechnologien (P42)

Appears in the scientific report 2011
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 Record created 2012-11-13, last modified 2018-02-10



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