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Journal Article | PreJuSER-45671 |
; ;
2005
IOP Publ.
Bristol
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Please use a persistent id in citations: http://hdl.handle.net/2128/23026 doi:10.1088/0953-8984/17/20/012
Abstract: The effective DNA-DNA interaction force is calculated by computer simulations with explicit tetravalent counterions and monovalent salt. For overcharged DNA molecules, the interaction force shows a double-minimum structure: The positions and depths of these minima are regulated by the counterion density in the bulk. Using two-dimensional lattice sums and free energy perturbation theories, the coexisting phases for DNA bundles are calculated. A DNA condensation and redissolution transition and a stable mesocrystal with an intermediate lattice constant for high counterion concentration are obtained.
Keyword(s): J
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