Journal Article PreJuSER-4948

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Does Cosmic-Ray-Induced Heterogeneous Chemistry Influence Stratospheric Polar Ozone Loss ?

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2009
APS College Park, Md.

Physical review letters 103, 228501 () [10.1103/PhysRevLett.103.228501]

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Abstract: Cosmic-ray (CR) -induced heterogeneous reactions of halogenated species have been suggested to play the dominant role in causing the Antarctic ozone hole. However, measurements of total ozone in Antarctica do not show a compact and significant correlation with CR activity. Further, a substantial CR-induced heterogeneous loss of chlorofluorocarbons is incompatible with multiyear satellite observations of N2O and CFC-12. Thus, CR-induced heterogeneous reactions cannot be considered as an alternative mechanism causing the Antarctic ozone hole.

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Note: We thank F. Rohrer for comments and for calculating the correlation coefficient of the data in Fig. 2 of Ref. [12]. ACE-FTS is funded by the Canadian Space Agency.

Research Program(s):
  1. Atmosphäre und Klima (P22)

Appears in the scientific report 2009
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 Record created 2012-11-13, last modified 2024-07-12


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