Journal Article PreJuSER-52292

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Chemical ozone loss in a chemistry-climate model from 1960 to 1999

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2006
American Geophysical Union Washington, DC

Geophysical research letters 33, L15820 () [10.1029/2006GL026939]

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Abstract: In the recent WMO assessment of ozone depletion, the minimum ozone column is used to assess the evolution of the polar ozone layer simulated in several chemistry-climate models (CCMs). The ozone column may be strongly influenced by changes in transport and is therefore not well-suited to identify changes in chemistry. The quantification of chemical ozone depletion can be achieved with tracer-tracer correlations (TRAC). For forty Antarctic winters ( 1960 - 1999), we present the seasonal chemical depletion simulated with the ECHAM4. L39(DLR)/CHEM model. Analyzing methane - ozone correlations, we find a mean chemical ozone loss of 80 +/- 10 DU during the 1990s, with a maximum of 94 DU. Compared to ozone loss deduced from HALOE measurements the model underestimates chemical loss by 37%. The average multidecadal trend in loss from 1960 to 1999 is 17 +/- 3 DU per decade. The largest contribution to this trend comes from the 62 +/- 11 DU ozone loss increase between the 1970s and 1990s.

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Note: Record converted from VDB: 12.11.2012

Contributing Institute(s):
  1. Stratosphäre (ICG-I)
  2. Jülich-Aachen Research Alliance - Simulation Sciences (JARA-SIM)
Research Program(s):
  1. Atmosphäre und Klima (P22)

Appears in the scientific report 2006
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 Record created 2012-11-13, last modified 2024-07-12