Journal Article FZJ-2016-02829

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Incommensurate spin correlations in highly oxidized cobaltates La$_{2−x}$Sr$_{x}$CoO$_{4}$

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2016
Nature Publishing Group London

Scientific reports 6, 25117 - () [10.1038/srep25117]

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Abstract: We observe quasi-static incommensurate magnetic peaks in neutron scattering experiments on layered cobalt oxides La2−xSrxCoO4 with high Co oxidation states that have been reported to be paramagnetic. This enables us to measure the magnetic excitations in this highly hole-doped incommensurate regime and compare our results with those found in the low-doped incommensurate regime that exhibit hourglass magnetic spectra. The hourglass shape of magnetic excitations completely disappears given a high Sr doping. Moreover, broad low-energy excitations are found, which are not centered at the incommensurate magnetic peak positions but around the quarter-integer values that are typically exhibited by excitations in the checkerboard charge ordered phase. Our findings suggest that the strong inter-site exchange interactions in the undoped islands are critical for the emergence of hourglass spectra in the incommensurate magnetic phases of La2−xSrxCoO4.

Classification:

Contributing Institute(s):
  1. Streumethoden (JCNS-2)
  2. Streumethoden (PGI-4)
  3. JARA-FIT (JARA-FIT)
  4. JCNS-ILL (JCNS-ILL)
Research Program(s):
  1. 144 - Controlling Collective States (POF3-144) (POF3-144)
  2. 524 - Controlling Collective States (POF3-524) (POF3-524)
  3. 6212 - Quantum Condensed Matter: Magnetism, Superconductivity (POF3-621) (POF3-621)
  4. 6213 - Materials and Processes for Energy and Transport Technologies (POF3-621) (POF3-621)
  5. 6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623) (POF3-623)
Experiment(s):
  1. PUMA: Thermal three axes spectrometer (SR7)
  2. PETRA Beamline P07 (PETRA III)

Appears in the scientific report 2016
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Medline ; Creative Commons Attribution CC BY 4.0 ; DOAJ ; OpenAccess ; BIOSIS Previews ; IF >= 5 ; JCR ; NCBI Molecular Biology Database ; SCOPUS ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection ; Zoological Record
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Dokumenttypen > Aufsätze > Zeitschriftenaufsätze
Institutssammlungen > JCNS > JCNS-ILL
JARA > JARA > JARA-JARA\-FIT
Institutssammlungen > JCNS > JCNS-2
Institutssammlungen > PGI > PGI-4
Workflowsammlungen > Öffentliche Einträge
Publikationsdatenbank
Open Access

 Datensatz erzeugt am 2016-06-01, letzte Änderung am 2025-01-29


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