Journal Article FZJ-2016-07345

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Solitary Magnons in the S = 5/2 Antiferromagnet CaFe$_2$O$_4$

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2016
APS College Park, Md.

Physical review letters 117(1), 017201 () [10.1103/PhysRevLett.117.017201]

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Abstract: CaFe2O4 is a S=52 anisotropic antiferromagnet based upon zig-zag chains having two competing magnetic structures, denoted as the A (↑↑↓↓) and B (↑↓↑↓) phases, which differ by the c-axis stacking of ferromagnetic stripes. We apply neutron scattering to demonstrate that the competing A and B phase order parameters result in magnetic antiphase boundaries along c which freeze on the time scale of ∼1  ns at the onset of magnetic order at 200 K. Using high resolution neutron spectroscopy, we find quantized spin wave levels and measure 9 such excitations localized in regions ∼1–2 c-axis lattice constants in size. We discuss these in the context of solitary magnons predicted to exist in anisotropic systems. The magnetic anisotropy affords both competing A+B orders as well as localization of spin excitations in a classical magnet.

Keyword(s): Magnetic Materials (1st) ; Magnetism (2nd)

Classification:

Contributing Institute(s):
  1. JCNS-FRM-II (JCNS (München) ; Jülich Centre for Neutron Science JCNS (München) ; JCNS-FRM-II)
  2. Streumethoden (JCNS-2)
Research Program(s):
  1. 6G15 - FRM II / MLZ (POF3-6G15) (POF3-6G15)
  2. 6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623) (POF3-623)
Experiment(s):
  1. DNS: Diffuse scattering neutron time of flight spectrometer (NL6S)

Appears in the scientific report 2016
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 Record created 2016-12-09, last modified 2021-01-29