Journal Article FZJ-2016-07390

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Conformational Properties of Active Semiflexible Polymers

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2016
MDPI Basel

Polymers 8(8), 304 () [10.3390/polym8080304]

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Abstract: The conformational properties of flexible and semiflexible polymers exposed to active noise are studied theoretically. The noise may originate from the interaction of the polymer with surrounding active (Brownian) particles or from the inherent motion of the polymer itself, which may be composed of active Brownian particles. In the latter case, the respective monomers are independently propelled in directions changing diffusively. For the description of the polymer, we adopt the continuous Gaussian semiflexible polymer model. Specifically, the finite polymer extensibility is taken into account, which turns out to be essential for the polymer conformations. Our analytical calculations predict a strong dependence of the relaxation times on the activity. In particular, semiflexible polymers exhibit a crossover from a bending elasticity-dominated dynamics to the flexible polymer dynamics with increasing activity. This leads to a significant activity-induced polymer shrinkage over a large range of self-propulsion velocities. For large activities, the polymers swell and their extension becomes comparable to the contour length. The scaling properties of the mean square end-to-end distance with respect to the polymer length and monomer activity are discussed

Classification:

Contributing Institute(s):
  1. Theorie der Weichen Materie und Biophysik (IAS-2)
  2. Theorie der Weichen Materie und Biophysik (ICS-2)
Research Program(s):
  1. 553 - Physical Basis of Diseases (POF3-553) (POF3-553)

Appears in the scientific report 2016
Database coverage:
Medline ; Creative Commons Attribution CC BY (No Version) ; DOAJ ; OpenAccess ; Current Contents - Physical, Chemical and Earth Sciences ; DOAJ Seal ; Ebsco Academic Search ; IF < 5 ; JCR ; SCOPUS ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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Dokumenttypen > Aufsätze > Zeitschriftenaufsätze
Institutssammlungen > IBI > IBI-5
Institutssammlungen > IAS > IAS-2
Workflowsammlungen > Öffentliche Einträge
ICS > ICS-2
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Open Access

 Datensatz erzeugt am 2016-12-12, letzte Änderung am 2024-06-10


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