Journal Article FZJ-2017-06834

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Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere

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2017
EGU Katlenburg-Lindau

Atmospheric chemistry and physics 17(11), 7055 - 7066 () [10.5194/acp-17-7055-2017]

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Abstract: Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i) into the tropical stratosphere (tropical pipe), and (ii) into the Northern Hemisphere (NH) extratropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5 % in the tropical pipe and 15 % in the extratropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN) and carbon monoxide (CO) observations, confirming that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the pollutants transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.

Classification:

Contributing Institute(s):
  1. Stratosphäre (IEK-7)
Research Program(s):
  1. 244 - Composition and dynamics of the upper troposphere and middle atmosphere (POF3-244) (POF3-244)

Appears in the scientific report 2017
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Medline ; Creative Commons Attribution CC BY 3.0 ; DOAJ ; OpenAccess ; Current Contents - Physical, Chemical and Earth Sciences ; DOAJ Seal ; IF >= 5 ; JCR ; NCBI Molecular Biology Database ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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 Record created 2017-10-04, last modified 2024-07-12