Journal Article FZJ-2017-08624

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The novel HALO mini-DOAS instrument: inferring trace gas concentrations from airborne UV/visible limb spectroscopy under all skies using the scaling method

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2017
Copernicus Katlenburg-Lindau

Atmospheric measurement techniques 10(11), 4209 - 4234 () [10.5194/amt-10-4209-2017]

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Abstract: We report on a novel six-channel optical spectrometer (further on called mini-DOAS instrument) for airborne nadir and limb measurements of atmospheric trace gases, liquid and solid water, and spectral radiances in the UV/vis and NIR spectral ranges. The spectrometer was developed for measurements from aboard the German High-Altitude and Long-Range (HALO) research aircraft during dedicated research missions. Here we report on the relevant instrumental details and the novel scaling method used to infer the mixing ratios of UV/vis absorbing trace gases from their absorption measured in limb geometry. The uncertainties of the scaling method are assessed in more detail than before for sample measurements of NO2 and BrO. Some first results are reported along with complementary measurements and comparisons with model predictions for a selected HALO research flight from Cape Town to Antarctica, which was performed during the research mission ESMVal on 13 September 2012.

Classification:

Contributing Institute(s):
  1. Stratosphäre (IEK-7)
  2. JARA - HPC (JARA-HPC)
Research Program(s):
  1. 244 - Composition and dynamics of the upper troposphere and middle atmosphere (POF3-244) (POF3-244)
  2. Chemisches Lagrangesches Modell der Stratosphäre(CLaMS) (jicg11_20160501) (jicg11_20160501)

Appears in the scientific report 2017
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Medline ; Creative Commons Attribution CC BY 3.0 ; DOAJ ; OpenAccess ; Current Contents - Physical, Chemical and Earth Sciences ; DOAJ Seal ; Ebsco Academic Search ; IF < 5 ; JCR ; SCOPUS ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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 Record created 2017-12-20, last modified 2024-07-12