Journal Article

FZJ-2018-02202

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png Partitioning of Lead and Lead Compounds under Gasification-Like Conditions

Bläsing, M. (Corresponding author)FZJ* ; Abascal, M. B. ; Ninomiya, Y. ; Müller, M.FZJ*

2018
American Chemical Society Columbus, Ohio

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Please use a persistent id in citations: doi:10.1021/acs.energyfuels.7b02803

Abstract: An investigation of the chemical form, the concentration, and distribution of lead species between the gas and condensed phase was carried out under gasification-like conditions. The influence of hydrogen sulfide, hydrogen chloride, and steam on the speciation of lead was studied. The gaseous species were determined online by molecular-beam-mass-spectrometry. The condensates were analyzed by standard methods. The dominant chemical forms were metallic Pb, PbCl2, and PbS. The experimental data were compared with the results of thermodynamic Scheil–Gulliver cooling calculations. Further, the experimental data was used as an input for a pseudoequilibrium model aiming at the determination of kinetic information on the underlying transformations.

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Contributing Institute(s):

1. Werkstoffstruktur und -eigenschaften (IEK-2)

Research Program(s):

1. 111 - Efficient and Flexible Power Plants (POF3-111) (POF3-111)

Appears in the scientific report 2018

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Database coverage:
; Current Contents - Engineering, Computing and Technology ; IF < 5 ; JCR ; NCBI Molecular Biology Database ; Nationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection

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