Journal Article FZJ-2019-02129

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Coexistence of Ferromagnetic and Stripe Antiferromagnetic Spin Fluctuations in SrCo$_2$As$_2$

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2019
APS College Park, Md.

Physical review letters 122(11), 117204 () [10.1103/PhysRevLett.122.117204]

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Abstract: We use inelastic neutron scattering to study energy and wave vector dependence of spin fluctuations in SrCo2As2, derived from SrFe2−xCoxAs2 iron pnictide superconductors. Our data reveal the coexistence of antiferromagnetic (AF) and ferromagnetic (FM) spin fluctuations at wave vectors QAF=(1,0) and QFM=(0,0)/(2,0), respectively. By comparing neutron scattering results with those of dynamic mean field theory calculation and angle-resolved photoemission spectroscopy experiments, we conclude that both AF and FM spin fluctuations in SrCo2As2 are closely associated with a flatband of the eg orbitals near the Fermi level, different from the t2g orbitals in superconducting SrFe2−xCoxAs2. Therefore, Co substitution in SrFe2−xCoxAs2 induces a t2g to eg orbital switching, and is responsible for FM spin fluctuations detrimental to the singlet pairing superconductivity.

Keyword(s): Magnetic Materials (1st) ; Magnetism (2nd)

Classification:

Contributing Institute(s):
  1. JCNS-FRM-II (JCNS-FRM-II)
  2. Streumethoden (JCNS-2)
Research Program(s):
  1. 6G15 - FRM II / MLZ (POF3-6G15) (POF3-6G15)
  2. 6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623) (POF3-623)
Experiment(s):
  1. Measurement at external facility

Appears in the scientific report 2019
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Institute Collections > JCNS > JCNS-FRM-II
Document types > Articles > Journal Article
Institute Collections > JCNS > JCNS-2
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 Record created 2019-03-26, last modified 2021-01-30