Journal Article FZJ-2019-06642

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Anisotropic spin fluctuations in detwinned FeSe

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2019
Nature Publishing Group Basingstoke

Nature materials 18(7), 709 - 716 () [10.1038/s41563-019-0369-5]

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Abstract: Superconductivity in FeSe emerges from a nematic phase that breaks four-fold rotational symmetry in the iron plane. This phase may arise from orbital ordering, spin fluctuations or hidden magnetic quadrupolar order. Here we use inelastic neutron scattering on a mosaic of single crystals of FeSe, detwinned by mounting on a BaFe2As2 substrate to demonstrate that spin excitations are most intense at the antiferromagnetic wave vectors QAF = (±1, 0) at low energies E = 6–11 meV in the normal state. This two-fold (C2) anisotropy is reduced at lower energies, 3–5 meV, indicating a gapped four-fold (C4) mode. In the superconducting state, however, the strong nematic anisotropy is again reflected in the spin resonance (E = 3.6 meV) at QAF with incommensurate scattering around 5–6 meV. Our results highlight the extreme electronic anisotropy of the nematic phase of FeSe and are consistent with a highly anisotropic superconducting gap driven by spin fluctuations.

Keyword(s): Magnetic Materials (1st) ; Condensed Matter Physics (2nd) ; Magnetism (2nd)

Classification:

Contributing Institute(s):
  1. JCNS-FRM-II (JCNS-FRM-II)
  2. Heinz Maier-Leibnitz Zentrum (MLZ)
Research Program(s):
  1. 6G15 - FRM II / MLZ (POF3-6G15) (POF3-6G15)
  2. 6212 - Quantum Condensed Matter: Magnetism, Superconductivity (POF3-621) (POF3-621)
  3. 6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623) (POF3-623)
Experiment(s):
  1. PANDA: Cold three axes spectrometer (SR2)
  2. PUMA: Thermal three axes spectrometer (SR7)

Appears in the scientific report 2019
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 Record created 2019-12-16, last modified 2021-01-30