Journal Article FZJ-2020-01692

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Spin Correlations and Short‐Range Magnetic Order in the Honeycomb‐Layered Na$_2$Ni$_2$TeO$_6$

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2020
Wiley-VCH Weinheim

Physica status solidi / B Basic research B 257(3), 1900232 () [10.1002/pssb.201900232]

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Abstract: An experimental study of long‐range magnetic order formation mechanisms in a layered structure with a honeycomb arrangement of the magnetic atoms Na2Ni2TeO6 is conducted. For the first time, the strong spin correlations are directly observed above the Neel temperature T N that is manifested in the presence of broad diffuse peaks on neutron diffraction patterns obtained with the XYZ polarization analysis. Due to the possibility of separating the magnetic, nuclear incoherent, and nuclear coherent contributions to the total neutron scattering cross section, it is unequivocally established that the observed diffuse scattering has magnetic nature. The spin‐pair correlation function is reconstructed by modeling diffuse neutron scattering on Na2Ni2TeO6 with reverse Monte Carlo method. The obtained results indicate 2D nature of the magnetic correlations, and moreover, the symmetry of short‐range magnetic state corresponds to long‐range zigzag‐type magnetic order in the honeycomb net, which is established earlier based on the theoretical calculations.

Keyword(s): Magnetic Materials (1st) ; Condensed Matter Physics (2nd)

Classification:

Contributing Institute(s):
  1. JCNS-FRM-II (JCNS-FRM-II)
  2. Streumethoden (JCNS-2)
  3. Heinz Maier-Leibnitz Zentrum (MLZ)
Research Program(s):
  1. 6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623) (POF3-623)
  2. 6G15 - FRM II / MLZ (POF3-6G15) (POF3-6G15)
Experiment(s):
  1. DNS: Diffuse scattering neutron time of flight spectrometer (NL6S)

Appears in the scientific report 2020
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Medline ; Embargoed OpenAccess ; Clarivate Analytics Master Journal List ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; IF < 5 ; JCR ; NationallizenzNationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Web of Science Core Collection
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Institutssammlungen > JCNS > JCNS-2
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Open Access

 Datensatz erzeugt am 2020-04-06, letzte Änderung am 2021-01-30


Published on 2019-07-12. Available in OpenAccess from 2020-07-12.:
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