Journal Article FZJ-2020-04931

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Orbital-enhanced warping effect in px,py-derived Rashba spin splitting of monatomic bismuth surface alloy

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2020
Nature Publishing Group [London]

npj quantum materials 5(1), 89 () [10.1038/s41535-020-00293-3]

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Abstract: Spin-split Rashba bands have been exploited to efficiently control the spin degree of freedom of moving electrons, which possesses a great potential in frontier applications of designing spintronic devices and processing spin-based information. Given an intrinsic breaking of inversion symmetry and sizeable spin–orbit interaction, two-dimensional (2D) surface alloys formed by heavy metal elements exhibit a pronounced Rashba-type spin splitting of the surface states. Here, we have revealed the essential role of atomic orbital symmetry in the hexagonally warped Rashba spin-split surface state of the 3–√×3–√R300 BiCu2 monatomic alloy by scanning tunneling spectroscopy (STS) and density functional theory (DFT). From dI/dU spectra and calculated band structures, three hole-like Rashba-split bands hybridized from distinct orbital symmetries have been identified in the unoccupied energy region. Because of the hexagonally deformed Fermi surface, quasi-particle interference (QPI) mappings have resolved scattering channels opened from interband transitions of px,py (mj = 1/2) band. In contrast to the s,pz-derived band, the hexagonal warping is predominately accompanied by substantial out-of-plane spin polarization Sz up to 24% in the dispersion of px,py (mj = 1/2) band with an in-plane orbital symmetry.

Classification:

Contributing Institute(s):
  1. Quanten-Theorie der Materialien (PGI-1)
  2. Quanten-Theorie der Materialien (IAS-1)
  3. JARA-FIT (JARA-FIT)
  4. JARA - HPC (JARA-HPC)
Research Program(s):
  1. 142 - Controlling Spin-Based Phenomena (POF3-142) (POF3-142)
  2. 143 - Controlling Configuration-Based Phenomena (POF3-143) (POF3-143)

Appears in the scientific report 2020
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Dokumenttypen > Aufsätze > Zeitschriftenaufsätze
JARA > JARA > JARA-JARA\-FIT
JARA > JARA > JARA-JARA\-HPC
Institutssammlungen > IAS > IAS-1
Institutssammlungen > PGI > PGI-1
Workflowsammlungen > Öffentliche Einträge
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Open Access

 Datensatz erzeugt am 2020-12-04, letzte Änderung am 2021-01-30


OpenAccess:
s41535-020-00293-3 - Volltext herunterladen PDF
2006.05024 - Volltext herunterladen PDF
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