Journal Article FZJ-2021-02157

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Soliton-Mediated Magnetic Reversal in an All-Oxide-Based Synthetic Antiferromagnetic Superlattice

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2021
Soc. Washington, DC

ACS applied materials & interfaces 13(17), 20788 - 20795 () [10.1021/acsami.1c02506]

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Abstract: All-oxide-based synthetic antiferromagnets (SAFs) are attracting intense research interest due to their superior tunability and great potentials for antiferromagnetic spintronic devices. In this work, using the La2/3Ca1/3MnO3/CaRu1/2Ti1/2O3 (LCMO/CRTO) superlattice as a model SAF, we investigated the layer-resolved magnetic reversal mechanism by polarized neutron reflectivity. We found that the reversal of LCMO layer moments is mediated by nucleation, expansion, and shrinkage of a magnetic soliton. This unique magnetic reversal process creates a reversed magnetic configuration of the SAF after a simple field cycling. Therefore, it can enable vertical data transfer from the bottom to the top of the superlattice. The physical origin of this intriguing magnetic reversal process could be attributed to the cooperation of the surface spin-flop effect and enhanced uniaxial magnetic anisotropy of the bottom LCMO layer. This work may pave a way to utilize all-oxide-based SAFs for three-dimensional spintronic devices with vertical data transfer and high-density data storage.

Keyword(s): Information and Communication (1st) ; Condensed Matter Physics (2nd) ; Magnetism (2nd)

Classification:

Contributing Institute(s):
  1. JCNS-FRM-II (JCNS-FRM-II)
  2. Heinz Maier-Leibnitz Zentrum (MLZ)
  3. Streumethoden (JCNS-2)
  4. JCNS-4 (JCNS-4)
Research Program(s):
  1. 6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ) (POF4-6G4) (POF4-6G4)
  2. 632 - Materials – Quantum, Complex and Functional Materials (POF4-632) (POF4-632)
Experiment(s):
  1. MARIA: Magnetic reflectometer with high incident angle (NL5N)
  2. Measurement at external facility

Appears in the scientific report 2021
Database coverage:
Medline ; Embargoed OpenAccess ; Clarivate Analytics Master Journal List ; Current Contents - Engineering, Computing and Technology ; Current Contents - Physical, Chemical and Earth Sciences ; Essential Science Indicators ; IF >= 5 ; JCR ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection
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Institute Collections > JCNS > JCNS-4
Institute Collections > JCNS > JCNS-2
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 Record created 2021-05-14, last modified 2022-02-21


Published on 2021-04-20. Available in OpenAccess from 2022-04-20.:
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