Journal Article FZJ-2021-02648

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Wall-anchored semiflexible polymer under large amplitude oscillatory shear flow

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2021
American Institute of Physics Melville, NY

The journal of chemical physics 154(22), 224901 () [10.1063/5.0051427]

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Abstract: The properties of semiflexible polymers tethered by one end to an impenetrable wall and exposed to oscillatory shear flow are investigated by mesoscale simulations. A polymer, confined in two dimensions, is described by a linear bead-spring chain, and fluid interactions are incorporated by the Brownian multiparticle collision dynamics approach. At small strain, the polymers follow the applied flow field. However, at high strain, we find a strongly nonlinear response with major conformational changes. Polymers are stretched along the flow direction and exhibit U-shaped conformations while following the flow. As a consequence of confinement in the half-space, frequency doubling in the time-dependent polymer properties appears along the direction normal to the wall

Classification:

Contributing Institute(s):
  1. Theoretische Physik der Lebenden Materie (IBI-5)
Research Program(s):
  1. 524 - Molecular and Cellular Information Processing (POF4-524) (POF4-524)

Appears in the scientific report 2021
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Medline ; Embargoed OpenAccess ; Clarivate Analytics Master Journal List ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; Essential Science Indicators ; IF < 5 ; JCR ; National-Konsortium ; NationallizenzNationallizenz ; PubMed Central ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection
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Open Access

 Datensatz erzeugt am 2021-06-17, letzte Änderung am 2024-06-10


Published on 2021-06-11. Available in OpenAccess from 2022-06-11.:
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