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Freezing of capillary waves at the glass transition

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2002
APS College Park, Md.

Physical review / B 65(18), 184207 () [10.1103/PhysRevB.65.184207]

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Abstract: The freezing of capillary waves on glycerol surfaces is studied by in situ x-ray reflectivity measurements. A wide temperature range around the calorimetric glass transition temperature at T(g)approximate to186 K is investigated. For T>250 K the obtained surface roughness as a function of the temperature differs significantly from the value predicted by the classical capillary waves theory. Below the temperature Tapproximate to250 K the magnitude of the roughness remains constant. Furthermore, a large hysteresis, i.e., a large difference of the roughnesses measured during cooling and heating of the sample, is observed. These findings are discussed in terms of viscosity effects.

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Note: Record converted from VDB: 12.11.2012

Contributing Institute(s):
  1. Streumethoden (IFF-STM)
Research Program(s):
  1. Kondensierte Materie (M02)

Appears in the scientific report 2002
Notes: This version is available at the following Publisher URL: http://prb.aps.org
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