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Magnetization dynamics in dysprosium orthoferrites via the inverse Faraday effect

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2006
APS College Park, Md.

Physical review / B 74(13), 134430 () [10.1103/PhysRevB.74.134430]

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Abstract: The ultrafast nonthermal control of magnetization has recently become feasible in canted antiferromagnets through photomagnetic instantaneous pulses [A. V. Kimel , Nature 435, 655 (2005)]. In this experiment, circularly polarized femtosecond laser pulses set up a strong magnetic field along the wave vector of the radiation through the inverse Faraday effect, thereby exciting nonthermally the spin dynamics of dysprosium orthoferrites. A theoretical study is performed by using a model for orthoferrites based on a general form of free energy whose parameters are extracted from experimental measurements. The magnetization dynamics is described by solving coupled sublattice Landau-Lifshitz-Gilbert equations whose damping term is associated with the scattering rate due to magnon-magnon interaction. Due to the inverse Faraday effect and the nonthermal excitation, the effect of the laser is simulated by magnetic-field Gaussian pulses with temporal width of the order of 100 fs. When the field is along the z axis, a single resonance mode of the magnetization is excited. The amplitude of the magnetization and out-of-phase behavior of the oscillations for fields in the z and -z directions are in good agreement with the cited experiment. The analysis of the effect of the temperature shows that the magnon-magnon scattering mechanism affects the decay of the oscillations on the picosecond scale. Finally, when the field pulse is along the x axis, another mode is excited, as observed in experiments. In this case, a comparison between theoretical and experimental results shows some discrepancies, the origin of which is related to the role played by anisotropies in orthoferrites.

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Research Program(s):
  1. Kondensierte Materie (P54)

Appears in the scientific report 2006
Notes: Nachtrag
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American Physical Society Transfer of Copyright Ag ; OpenAccess
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