Journal Article

FZJ-2019-04404

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png The impact of recent changes in Asian anthropogenic emissions of SO₂ on sulfate loading in the upper troposphere and lower stratosphere and the associated radiative changes

Fadnavis, S. (Corresponding author) ; Müller, R.FZJ* ; Kalita, G. ; Rowlinson, M. ; Rap, A. ; Li, J. F. ; Gasparini, B. ; Laakso, A.

2019
EGU Katlenburg-Lindau

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Please use a persistent id in citations: http://hdl.handle.net/2128/22818  doi:10.5194/acp-19-9989-2019

Abstract: Convective transport plays a key role in aerosol enhancement in the upper troposphere and lower stratosphere (UTLS) over the Asian monsoon region where low-level convective instability persists throughout the year. We use the state-of-the-art ECHAM6–HAMMOZ global chemistry–climate model to investigate the seasonal transport of anthropogenic Asian sulfate aerosols and their impact on the UTLS. Sensitivity simulations for SO2 emission perturbation over India (48 % increase) and China (70 % decrease) are performed based on the Ozone Monitoring Instrument (OMI) satellite-observed trend, rising over India by ∼4.8 % per year and decreasing over China by ∼7.0 % per year during 2006–2017. The enhanced Indian emissions result in an increase in aerosol optical depth (AOD) loading in the UTLS by 0.61 to 4.17 % over India. These aerosols are transported to the Arctic during all seasons by the lower branch of the Brewer–Dobson circulation enhancing AOD by 0.017 % to 4.8 %. Interestingly, a reduction in SO2 emission over China inhibits the transport of Indian sulfate aerosols to the Arctic in summer-monsoon and post-monsoon seasons due to subsidence over northern India. The region of sulfate aerosol enhancement shows significant warming in the UTLS over northern India, south China (0.2±0.15 to 0.8±0.72 K) and the Arctic (∼1±0.62 to 1.6±1.07 K). The estimated seasonal mean direct radiative forcing at the top of the atmosphere (TOA) induced by the increase in Indian SO2 emission is −0.2 to −1.5 W m−2 over northern India. The Chinese SO2 emission reduction leads to a positive radiative forcing of ∼0.6 to 6 W m−2 over China. The decrease in vertical velocity and the associated enhanced stability of the upper troposphere in response to increased Indian SO2 emissions will likely decrease rainfall over India.

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Contributing Institute(s):

1. Stratosphäre (IEK-7)

Research Program(s):

1. 244 - Composition and dynamics of the upper troposphere and middle atmosphere (POF3-244) (POF3-244)

Appears in the scientific report 2019

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Database coverage:
; ; ; ; Clarivate Analytics Master Journal List ; Current Contents - Physical, Chemical and Earth Sciences ; DOAJ Seal ; IF >= 5 ; JCR ; NCBI Molecular Biology Database ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Web of Science Core Collection

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