Journal Article

FZJ-2020-00104

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png Separation of Carbon Dioxide from Real Power Plant Flue Gases by Gas Permeation Using a Supported Ionic Liquid Membrane: An Investigation of Membrane Stability

Klingberg, P. (Corresponding author) ; Wilkner, K.FZJ* ; Schlüter, M. ; Grünauer, J. ; Shishatskiy, S.

2019
MDPI Basel

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Please use a persistent id in citations: http://hdl.handle.net/2128/23820  doi:10.3390/membranes9030035

Abstract: The separation of carbon dioxide from coal-fired power plant flue gases using a CO2/N2-selective supported ionic liquid membrane (SILM) was investigated and the performance and stability of the membrane during operation are reported. The membrane is composed of a polyacrylonitrile (PAN) ultrafiltration membrane as a support and a selective layer of an ionic liquid (IL), 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMIM Tf2N). The feasibility of large-scale SILM production was demonstrated by the formation of a square-meter-scale membrane and preparation of a membrane module. A flat-sheet envelope-type SILM module containing 0.67 m2 of the membrane was assembled. Prior to real flue gas operation, the separation behaviour of the membrane was investigated with single gases. The stability of the SILM during the test stand and pilot plant operation using real power plant flue gases is reported. The volume fraction of carbon dioxide in the flue gas was raised from approx. 14 vol. % (feed) to 40 vol. % (permeate). However, issues concerning the membrane stability were found when SO3 aerosols in large quantities were present in the flue gas

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Contributing Institute(s):

1. Werkstoffsynthese und Herstellungsverfahren (IEK-1)

Research Program(s):

1. 113 - Methods and Concepts for Material Development (POF3-113) (POF3-113)

Appears in the scientific report 2019

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Database coverage:
; ; ; ; Clarivate Analytics Master Journal List ; DOAJ Seal ; Ebsco Academic Search ; Emerging Sources Citation Index ; NCBI Molecular Biology Database ; PubMed Central ; SCOPUS ; Web of Science Core Collection

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