Journal Article FZJ-2020-01727

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Dehydration and low ozone in the tropopause layer over the Asian monsoon caused by tropical cyclones: Lagrangian transport calculations using ERA-Interim and ERA5 reanalysis data

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2020
EGU Katlenburg-Lindau

Atmospheric chemistry and physics 20(7), 4133 - 4152 () [10.5194/acp-20-4133-2020]

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Abstract: Low ozone and high water vapour mixing ratios are common features in the Asian summer monsoon (ASM) anticyclone; however, low ozone and low water vapour values were observed near the tropopause over Kunming, China, within the ASM using balloon-borne measurements performed during the SWOP (sounding water vapour, ozone, and particle) campaign in August 2009 and 2015. Here, we investigate low ozone and water vapour signatures in the upper troposphere and lower stratosphere (UTLS) using FengYun-2D, FengYun-2G, and Aura Microwave Limb Sounder (MLS) satellite measurements and backward trajectory calculations. Trajectories with kinematic and diabatic vertical velocities were calculated using the Chemical Lagrangian Model of the Stratosphere (CLaMS) trajectory module driven by both ERA-Interim and ERA5 reanalysis data.All trajectory calculations show that air parcels with low ozone and low water vapour values in the UTLS over Kunming measured by balloon-borne instruments originate from the western Pacific boundary layer. Deep convection associated with tropical cyclones over the western Pacific transports ozone-poor air from the marine boundary layer to the cold tropopause region. Subsequently, these air parcels are mixed into the strong easterlies on the southern side of the Asian summer monsoon anticyclone. Air parcels are dehydrated when passing the lowest temperature region (< 190 K) at the convective outflow of tropical cyclones. However, trajectory calculations show different vertical transport via deep convection depending on the employed reanalysis data (ERA-Interim, ERA5) and vertical velocities (diabatic, kinematic). Both the kinematic and the diabatic trajectory calculations using ERA5 data show much faster and stronger vertical transport than ERA-Interim primarily because of ERA5's better spatial and temporal resolution, which likely resolves convective events more accurately. Our findings show that the interplay between the ASM anticyclone and tropical cyclones has a significant impact on the chemical composition of the UTLS during summer.

Classification:

Contributing Institute(s):
  1. Stratosphäre (IEK-7)
Research Program(s):
  1. 244 - Composition and dynamics of the upper troposphere and middle atmosphere (POF3-244) (POF3-244)

Appears in the scientific report 2020
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Medline ; Creative Commons Attribution CC BY 4.0 ; DOAJ ; OpenAccess ; Clarivate Analytics Master Journal List ; Current Contents - Physical, Chemical and Earth Sciences ; DOAJ Seal ; IF >= 5 ; JCR ; NCBI Molecular Biology Database ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Web of Science Core Collection
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 Record created 2020-04-10, last modified 2024-07-12