Journal Article FZJ-2021-04858

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a -axis YBa 2 Cu 3 O 7− x /PrBa 2 Cu 3 O 7− x /YBa 2 Cu 3 O 7− x trilayers with subnanometer rms roughness

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2021
AIP Publ. Melville, NY

APL materials 9(2), 021117 - () [10.1063/5.0034648]

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Abstract: We demonstrate a-axis YBa 2 Cu 3 O 7−x /PrBa 2 Cu 3 O 7−x /YBa 2 Cu 3 O 7−x trilayers grown on (100) LaAlO 3 substrates with improved interfacesmoothness. The trilayers are synthesized by ozone-assisted molecular-beam epitaxy. The thickness of the PrBa 2 Cu 3 O 7−x layer is held con-stant at 8 nm, and the thickness of the YBa 2 Cu 3 O 7−x layers is varied from 24 nm to 100 nm. X-ray diffraction measurements show all trilayersto have >97% a-axis content. The rms roughness of the thinnest trilayer is <0.7 nm, and this roughness increases with the thickness of theYBa 2 Cu 3 O 7−x layers. The thickness of the YBa 2 Cu 3 O 7−x layers also affects the transport properties: while all samples exhibit an onset of thesuperconducting transition at and above 85 K, the thinner samples show wider transition widths, ΔT c . High-resolution scanning transmissionelectron microscopy reveals coherent and chemically sharp interfaces and that growth begins with a cubic (Y,Ba)CuO 3−x perovskite phase thattransforms into a-axis oriented YBa 2 Cu 3 O 7−x as the substrate temperature is ramped up.

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Contributing Institute(s):
  1. Halbleiter-Nanoelektronik (PGI-9)
Research Program(s):
  1. 5233 - Memristive Materials and Devices (POF4-523) (POF4-523)

Appears in the scientific report 2021
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 Record created 2021-12-02, last modified 2022-01-03


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