Journal Article FZJ-2021-04861

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Engineering new limits to magnetostriction through metastability in iron-gallium alloys

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2021
Nature Publishing Group UK [London]

Nature Communications 12(1), 2757 () [10.1038/s41467-021-22793-x]

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Abstract: Magnetostrictive materials transduce magnetic and mechanical energies and when combinedwith piezoelectric elements, evoke magnetoelectric transduction for high-sensitivity magneticfield sensors and energy-efficient beyond-CMOS technologies. The dearth of ductile, rare-earth-free materials with high magnetostrictive coefficients motivates the discovery ofsuperior materials. Fe 1−x Ga x alloys are amongst the highest performing rare-earth-freemagnetostrictive materials; however, magnetostriction becomes sharply suppressed beyondx = 19% due to the formation of a parasitic ordered intermetallic phase. Here, we harnessepitaxy to extend the stability of the BCC Fe 1−x Ga x alloy to gallium compositions as high asx = 30% and in so doing dramatically boost the magnetostriction by as much as 10x relativeto the bulk and 2x larger than canonical rare-earth based magnetostrictors. A Fe 1−x Ga x − [Pb(Mg 1/3 Nb 2/3 )O 3 ] 0.7 −[PbTiO 3 ] 0.3 (PMN-PT) composite magnetoelectric shows robust 90°electrical switching of magnetic anisotropy and a converse magnetoelectric coefficientof 2.0 × 10 −5 s m −1 . When optimally scaled, this high coefficient implies stable switching at~80 aJ per bit.

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Contributing Institute(s):
  1. Halbleiter-Nanoelektronik (PGI-9)
Research Program(s):
  1. 5233 - Memristive Materials and Devices (POF4-523) (POF4-523)

Appears in the scientific report 2021
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 Record created 2021-12-02, last modified 2022-01-03


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