Journal Article

FZJ-2023-05469

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png Understanding Battery Interfaces by Combined Characterizationand Simulation Approaches: Challenges and Perspectives

Duncan, A. ; Elixabete, A. ; Benayad, A. ; Capone, F. G. ; Enio, C. ; Ivano, C. E. ; Cekic-Laskovic, I.FZJ* ; Raul, C. ; Dudy, L. ; Edström, K. ; Johnson, M. R. ; Li, H. ; Lastra, J. M. G. ; Souza, M. L. D. ; Meunier, V. ; Morcrette, M. ; Reichert, H. ; Simon, P. ; Rueff, J.-P. ; Sottmann, J. ; Wenzel, W. (Corresponding author) ; Grimaud, A. (Corresponding author)

2022
Wiley-VCH Weinheim

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Please use a persistent id in citations: doi:10.1002/aenm.202102687  doi:10.34734/FZJ-2023-05469

Abstract: Driven by the continuous search for improving performances, understandingthe phenomena at the electrode/electrolyte interfaces has become an overridingfactor for the success of sustainable and efficient battery technologiesfor mobile and stationary applications. Toward this goal, rapid advances havebeen made regarding simulations/modeling techniques and characterizationapproaches, including high-throughput electrochemical measurementscoupled with spectroscopies. Focusing on Li-ion batteries, current developmentsare analyzed in the field as well as future challenges in order to gaina full description of interfacial processes across multiple length/timescales;from charge transfer to migration/diffusion properties and interphases formation,up to and including their stability over the entire battery lifetime. Forsuch complex and interrelated phenomena, developing a unified workflowintimately combining the ensemble of these techniques will be critical tounlocking their full investigative potential. For this paradigm shift in batterydesign to become reality, it necessitates the implementation of researchstandards and protocols, underlining the importance of a concerted approachacross the community. With this in mind, major collaborative initiatives gatheringcomplementary strengths and skills will be fundamental if societal andenvironmental imperatives in this domain are to be met.

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Contributing Institute(s):

1. Helmholtz-Institut Münster Ionenleiter für Energiespeicher (IEK-12)

Research Program(s):

1. 1222 - Components and Cells (POF4-122) (POF4-122)
2. BIG-MAP - Battery Interface Genome - Materials Acceleration Platform (957189) (957189)
3. BATTERY 2030PLUS - BATTERY 2030+ large-scale research initiative: At the heart of a connected green society (957213) (957213)

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Database coverage:
; ; ; Clarivate Analytics Master Journal List ; Current Contents - Engineering, Computing and Technology ; Current Contents - Physical, Chemical and Earth Sciences ; DEAL Wiley ; Ebsco Academic Search ; Essential Science Indicators ; IF >= 25 ; JCR ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection

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