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Journal Article | FZJ-2024-05163 |
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2024
Nature Publishing Group
London [u.a.]
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Please use a persistent id in citations: doi:10.1038/s41565-024-01724-z doi:10.34734/FZJ-2024-05163
Abstract: The detection of faint magnetic fields from single-electron and nuclear spinsat the atomic scale is a long-standing challenge in physics. While currentmobile quantum sensors achieve single-electron spin sensitivity, atomicspatial resolution remains elusive for existing techniques. Here we fabricate asingle-molecule quantum sensor at the apex of the metallic tip of a scanningtunnelling microscope by attaching Fe atoms and a PTCDA (3,4,9,10-perylenetetracarboxylic-dianhydride) molecule to the tip apex. We address themolecular spin by electron spin resonance and achieve ~100 neV resolutionin energy. In a proof-of-principle experiment, we measure the magnetic andelectric dipole fields emanating from a single Fe atom and an Ag dimer on anAg(111) surface with sub-angstrom spatial resolution. Our method enablesatomic-scale quantum sensing experiments of electric and magnetic fields onconducting surfaces and may find applications in the sensing of spin-labelledbiomolecules and of spin textures in quantum materials.
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