Journal Article FZJ-2020-04272

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Photoemission electron microscopy of magneto-ionic effects in La0.7Sr0.3MnO3

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2020
AIP Publ. Melville, NY

APL materials 8(11), 111102 () [10.1063/5.0022150]

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Abstract: Magneto-ionic control of magnetism is a promising route toward the realization of non-volatile memory and memristive devices. Magneto-ionic oxides are particularly interesting for this purpose, exhibiting magnetic switching coupled to resistive switching, with the latter emerging as a perturbation of the oxygen vacancy concentration. Here, we report on electric-field-induced magnetic switching in a La0.7Sr0.3MnO3 (LSMO) thin film. Correlating magnetic and chemical information via photoemission electron microscopy, we show that applying a positive voltage perpendicular to the film surface of LSMO results in the change in the valence of the Mn ions accompanied by a metal-to-insulator transition and a loss of magnetic ordering. Importantly, we demonstrate that the voltage amplitude provides granular control of the phenomena, enabling fine-tuning of the surface electronic structure. Our study provides valuable insight into the switching capabilities of LSMO that can be utilized in magneto-ionic devices.

Classification:

Contributing Institute(s):
  1. Elektronische Eigenschaften (PGI-6)
  2. Elektronische Materialien (PGI-7)
  3. Streumethoden (JCNS-2)
  4. Streumethoden (PGI-4)
  5. JARA-FIT (JARA-FIT)
  6. Jülich-Aachen Research Alliance - Fundamentals of Future Information Technology (JARA-FIT)
Research Program(s):
  1. 522 - Controlling Spin-Based Phenomena (POF3-522) (POF3-522)
  2. DFG project 167917811 - SFB 917: Resistiv schaltende Chalkogenide für zukünftige Elektronikanwendungen: Struktur, Kinetik und Bauelementskalierung "Nanoswitches" (167917811) (167917811)

Appears in the scientific report 2020
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Document types > Articles > Journal Article
Institute Collections > JCNS > JCNS-2
JARA > JARA > JARA-JARA\-FIT
Institute Collections > PGI > PGI-6
Institute Collections > PGI > PGI-7
Institute Collections > PGI > PGI-4
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 Record created 2020-11-04, last modified 2025-01-29