Journal Article FZJ-2020-05235

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Dynamical diffraction effects in STEM orbital angular momentum resolved electron energy-loss magnetic chiral dichroism

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2020
Inst. Woodbury, NY

Physical review / B 102(18), 184420 () [10.1103/PhysRevB.102.184420]

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Abstract: In this paper, we explore the properties of dynamical diffraction coefficients in orbital angular momentum resolved electron energy-loss magnetic chiral dichroism spectra, in a scanning transmission electron microscopy setup. We demonstrate that for basic zone axis geometries with fourfold or threefold symmetry the coefficients are constrained to have simplified forms. By exploiting these properties, we show how a dichroism spectrum accessible using this technique is only weakly dependent on sample thickness and, more generally, on dynamical diffraction effects. Our results indicate that in such cases it is possible to determine the orbital and spin components of atomic magnetic moments approximately from experimental spectra without the need for additional dynamical diffraction calculations.

Classification:

Contributing Institute(s):
  1. Physik Nanoskaliger Systeme (ER-C-1)
Research Program(s):
  1. 143 - Controlling Configuration-Based Phenomena (POF3-143) (POF3-143)
  2. Q-SORT - QUANTUM SORTER (766970) (766970)
  3. 3D MAGiC - Three-dimensional magnetization textures: Discovery and control on the nanoscale (856538) (856538)
  4. ESTEEM3 - Enabling Science and Technology through European Electron Microscopy (823717) (823717)
  5. DARPA, Phase 2 - Defense Advanced Research Projects Agency Manipulation of magnetic skyrmions for logicin- memory applications (Z1422.01.18) (Z1422.01.18)
  6. DFG project 405553726 - TRR 270: Hysterese-Design magnetischer Materialien für effiziente Energieumwandlung (405553726) (405553726)

Appears in the scientific report 2020
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 Record created 2020-12-14, last modified 2023-04-26


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